Catalytic alkylation of remote C–H bonds enabled by proton-coupled electron transfer

Catalytic alkylation of remote C–H bonds enabled by proton-coupled electron transfer
Gilbert J. Choi, Qilei Zhu, David C. Miller, Carol J. Gu & Robert R. Knowles

Catalytic alkylation of C–H bonds is achieved via homolysis of N–H bonds of N-alkyl amides through proton-coupled electron transfer.

Nature 539, 268–271 (10 November 2016) doi:10.1038/nature19811

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